Persistent Photoconductivity in Monolayer MoS$_{2}$ on Organic-molecule-functionalized Substrates

ORAL

Abstract

We demonstrate a giant persistent photoconductivity (PPC) effect in monolayer MoS$_{2}$ in which the photocurrent robustly persists after illumination has ceased. This PPC effect in monolayer MoS$_{2}$ on organic-molecule-functionalized substrates sustains up to room temperature and can be highly suppressed by applying source--drain/back-gate voltages to the transistors. Based on this persistency and controllability of the PPC effect, we achieve a room-temperature conductance bistability by utilizing optical and electrical pulses. The observed giant PPC effect in MoS$_{2}$ can be attributed to a large electron-capture barrier of trap states, which is estimated to be as high as 390 meV.

Authors

  • Wei-Hua Wang

    • Institute of Atomic and Molecular Sciences, Academia Sinica
  • Yueh-Chun Wu

    • Institute of Atomic and Molecular Sciences, Academia Sinica
  • Shao-Yu Chen

    • Institute of Atomic and Molecular Sciences, Academia Sinica
  • Cheng-Hua Liu

    • Department of Physics, National Taiwan University
  • Po-Hsun Ho

    • Department of Materials Science and Engineering, National Taiwan University
  • Chun-Wei Chen

    • Department of Materials Science and Engineering, National Taiwan University
  • Chi-Te Liang

    • Department of Physics, National Taiwan University