Magnetic excitations in spin-orbital liquid FeSc$_2$S$_4$ in zero and applied magnetic field probed by inelastic neutron scattering

ORAL

Abstract

In systems where both spin and orbital frustration are present, an intriguing Spin Orbital Liquid (SOL) state is believed to occur where spin and orbital moments remain disordered down to the lowest measurable temperatures. The A-site spinel FeSc$_2$S$_4$ is believed to form such a SOL ground state, with its undistorted cubic structure and diamond lattice of Fe$^{2+}$ sites providing the ingredients for orbital and spin frustration, respectively. The system displays Curie-Weiss behaviour indicative of strong exchange between $S=2$, $L=2$ Fe$^{2+}$ ions, though it does not order down to the lowest measurable temperatures. Here I will present the results of inelastic, time-of-flight neutron scattering experiments that probe the full bandwidth of the magnetic excitations in a powder sample of FeSc$_2$S$_4$, and provide a consistent model of the observed dynamics in terms of spin-orbital excitations, in both zero-field and in-field measurements. I will discuss in particular how the application of a magnetic field elucidates the spin and orbital nature of these excitations, as the system shows behaviour drastically contrary to its spin-only analogue.

*We acknowledge support from EPSRC (UK)

Authors

  • Alun Biffin

    • University of Oxford
  • Radu Coldea

    • University of Oxford
    • University of Oxford, UK
    • Clarendon Laboratory, Department of Physics, University of Oxford, Oxford OX1 3PU, United Kingdom
  • Christian R\"{u}egg

    • Paul Scherrer Institute and University of Geneva, Switzerland
    • Paul Scherrer Institut
  • Oksana Zaharko

    • Paul Scherrer Institut
  • Jan Embs

    • Paul Scherrer Institut
  • Tatiana Guidi

    • ISIS at Rutherford Appleton Laboratory
  • Vladimir Tsurkan

    • Universit\"{a}t Augburg