Observation of negative terahertz photoconductivity in monolayer MoS$_{2}$ under femtosecond laser excitation

ORAL

Abstract

We observed a pronounced transient decrease of terahertz conductivity in doped monolayer molybdenum disulfide (MoS$_{2})$ after pulsed laser excitation. This anomalous phenomenon arises from the strong many-body interactions in the system, where optically produced electron-hole pairs join the doped charges to form trions, bound states of two electrons and one hole, and substantially diminish the carrier conductivity by the resulting increase of effective mass. Our results reveal the ultrafast formation and decay of trions in monolayer MoS$_{2}$ and their influence on the conductivity of the material.

Authors

  • Chun Hung Lui

    • Columbia University
    • Massachusetts Institute of Technology
  • Alex J. Frenzel

    • Massachusetts Institute of Technology
  • Daniel V. Pilon

    • Massachusetts Institute of Technology
  • Yi-Hsien Lee

    • Massachusetts Institute of Technology
  • Jing Kong

    • Massachusetts Institute of Technology, Boston, MA, USA
    • Massachussetts Institute of Technology
    • MIT EECS
    • Massachusetts Institute of Technology
  • Nuh Gedik

    • Massachusetts Institute of Technology