The Angular Dependent Magnetic Phase Diagram of Cs$_{2}$CuCl$_{4}$

ORAL

Abstract

We present a determination of the phase diagram of the $S = {1\over2}$ quasi-2D triangular Heisenberg quantum antiferromagnet Cs$_{2}$CuCl$_{4}$ at temperatures to down 100mK and fields up to the saturation field of 9 tesla. We have determined the low temperature phase boundaries as a function of angle to the magnetic field using a unique low temperature rotatable calorimeter. Measurements at several angles intermediate to the in-plane and perpendicular directions elucidate the evolution of the complex phase diagram between these two principal axis. For fields directed along the a-axis (perpendicular to the plane of the triangular lattice), we observe a series of magnetic phases. New, unexpected phases arise at intermediate angles as we rotate the magnetic field away from the a-axis, into the bc plane. Variation of phase boundaries with field angle within the bc plane reflect interactions due to the Dzyaloshinskii-Moriya mechanism.

*A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement No. DMR-1157490, the State of Florida, and the U.S. Department of Energy.

Authors

  • Scott Hannahs

    • National High Magnetic Field Lab, Tallahassee, FL
    • National High Magnetic Field Laboratory
  • Nathanael Fortune

    • Department of Physics, Smith College, Northampton, MA
    • Department of Physics, Smith College
  • Yasumasa Takano

    • Department of Physics, University of Florida, Gainesville, FL
    • Department of Physics, University of Florida
  • Toshio Ono

    • Department of Physics, Osaka Prefecture University, Osaka
  • Hidekazu Tanaka

    • Department of Physics, Tokyo Institute of Technology, Meguro-ku, Tokyo