Magnetic Excitations in MnV$_{2}$O$_{4}$ Studied by Inelastic Neutron Scattering

ORAL

Abstract

We focus on the dynamical structure of a spin-orbital coupled system MnV$_{2}$O$_{4}$, which crystallizes in the spinel structure. Each V$^{3+}$ ion with the 3d$^{2}$ configuration is surrounded by an oxygen octahedron. The orbital degree of freedom consequently exists in the t$_{\mathrm{2g}}$ states. Below T$_{\mathrm{oo}}=$53K, the t$_{\mathrm{2g}}$ orbitals are arranged in the layered antiferroic way. Simultaneously, non-collinear ferrimagnetic ordering takes place. In this spin-orbital correlated system, in addition to conventional spin waves, orbital waves and spin-orbital coupled excitations are expected to appear. A measurement of inelastic neutron scattering on single crystals of MnV$_{2}$O$_{4}$ was carried out at 5K using a Fermi-chopper type spectrometer 4SEASONS installed at BL01, J-PARC, Japan. The dispersion of the magnetic excitations at 8-9meV have been revealed, which was only rather vaguely observed in the previous study. We have performed spin-wave calculations based on the spin Hamiltonian and compared with the experimental results in order to identify the 8-9meV modes.

Authors

  • Keisuke Matsuura

    • Department of Advanced Materials Science, The University of Tokyo, Kashiwa 277-8561, Japan
  • Amane Uehara

    • Department of Applied Physics, The University of Tokyo, Hongo, Tokyo 113-8656, Japan
  • Yoichi Nii

    • Department of Advanced Materials Science, The University of Tokyo, Kashiwa 277-8561, Japan
  • Nobuyuki Abe

    • Department of Advanced Materials Science, The University of Tokyo, Kashiwa 277-8561, Japan
  • Hajime Sagayama

    • Department of Advanced Materials Science, The University of Tokyo, Kashiwa 277-8561, Japan
  • Taka-hisa Arima

    • Department of Advanced Materials Science, The University of Tokyo, Kashiwa 277-8561, Japan
  • Sungdae Ji

    • Research Center for Neutron Science and Technology, Comprehensive Research Organaization for Science and Society, Tokai, Ibaraki 319-1106, Japan
  • Ryoichi Kajimoto

    • Research Center for Neutron Science and Technology, Comprehensive Research Organaization for Science and Society, Tokai, Ibaraki 319-1106, Japan