Iridate compound produces extraordinarily high coercive magnetic field

ORAL

Abstract

We present a data on an iridate compound that shows an extraordinarily large magnetic hysteresis loop. The coercive magnetic field exceeds 40 Tesla in single-crystal samples. The hysteresis coexists with a linear background, and the total remanent magnetization is about half a Bohr magneton. We will discuss the emergence of these properties from the interplay of spin-orbit coupling, magnetic exchange and possible frustration. The single crystalline material exhibits a magnetic hysteresis loop for one orientation of the magnetic field and a smooth linear increase in the magnetization with field for the other. Measurements were conducted in 65 T short-pulse magnets and the 60 Tesla shaped-pulse magnet at the National High Magnetic Field Lab in Los Alamos. We do not observe any dependence of the magnetic hysteresis on magnetic field sweep rate. Compounds containing Ir4$+$ have attracted attention recently due to strong spin-orbit coupling that competes with crystal-electric field and exchange interactions. This competition can result in non-Hund's-rule ground states with unusual properties.

Authors

  • Vivien Zapf

    • National High Magnetic Field Lab
    • Los Alamos National laboratory, Los Alamos, NM, 87544, USA
    • National High Magnetic Field Lab (NHMFL), Los Alamos National Lab (LANL)
  • Craig Topping

    • U. Edinburgh, UK
  • Jae-Wook Kim

    • NHMFL, LANL
  • Eun-Deok Mun

    • Ames Lab
  • Paul Goddard

    • Oxford U., UK
  • Saman Ghannadzadeh

    • Oxford U., UK
  • Xuan Luo

    • POSTECH, Korea
  • Sang-Wook Cheong

    • Rutgers Center for Emergent Materials \& Dept of Physics, Rutgers University
  • John Singleton

    • NHMFL, LANL