Synthesis, structure and magnetic properties of BaFe$_{2}$(As$_{\mathrm{1-x}}$P$_{\mathrm{x}}$)$_{2}$ as determined by elastic and inelastic neutron scattering

ORAL

Abstract

Unconventional superconductivity and microscopic phase coexistence have been demonstrated in a narrow compositional region of the122 system between two competing spin density wave and superconducting order parameters. Quantum critical fluctuations induced by the suppression of the antiferromagnetic order have been proposed to mediate pairing in analogy with the role played by phonons in conventional cuprates. Establishing unambiguous conclusions concerning the pairing mechanism has proven difficult in the pnictides due to the complexity of the electronic structures. Recent reports have shown that isovalent P substitution for As in BaFe$_{2}$As$_{2}$ suppresses the structural and magnetic transitions and lead to superconductivity similar to hole or electron doping. From the chemical point-of-view, there is no net change in the electron-to-hole ratio in this charge compensated system. I will briefly discuss synthesis details of high quality pnictides and BaFe$_{2}$(As$_{\mathrm{1-x}}$P$_{\mathrm{x}}$)$_{2}$ samples and present structural results obtained by neutron diffraction. Inelastic neutron measurements will also be discussed.

Authors

  • Keith M. Taddei

    • Northern Illinois University
  • J.M. Allred

    • Argonne National Lab
    • Argonne National Laboratory (ANL)
  • R. Osborn

    • Argonne National Laboratory
    • Argonne National Laboratory (ANL)
    • ANL
  • S. Rosenkranz

    • Argonne National Lab
    • Argonne National Laboratory (ANL)
    • ANL
  • D. Bugaris

    • Argonne National Lab
    • Argonne National Laboratory (ANL)
  • H. Claus

    • Argonne National Laboratory (ANL)
  • M. Kanatzidis

    • Department of Chemistry, Northwestern University, Evaston, Illinois 60208, USA
    • Northwestern University
    • Argonne National Laboratory and Northwestern University
    • Argonne National Laboratory; Northwestern University
    • ANL and Northwestern University
  • S. Avci

    • Bursa Technical University and Argonne National Laboratory
    • Bursa technical University, Turkey
  • C. de la Cruz

    • Oak Ridge National Lab
    • Oak Ridge National Laboratory
  • Omar Chmaissem

    • Argonne National Laboratory, Northern Illinois University
    • Department of Physics, Northern Illinois University, De Kalb, IL 60115
    • Argonne National Lab
    • Northern Illinois University and ANL
    • Northern Illinois University and Argonne National Laboratory (ANL)