Microscopic Evidence for Slater-Type Metal-Insulator Transition in Sr$_{2}$IrO$_{4}$

ORAL

Abstract

The interplay between spin-orbit coupling, bandwidth and on-site coulomb repulsion in layered 5d transition metal oxides (TMO) acquired much interest recently. In Sr$_{2}$IrO$_{4}$, the interplay opens a gap near the Fermi energy and stabilizes a J$_{\mathrm{eff}}=$1/2 spin-orbital entangled insulating state at low temperatures. However, whether this metal-insulating transition (MIT) is Mott-type (electronic-correlation driven) or slater-type (magnetic order driven) is still under hot debate. In this presentation, we give, for the first time, the atomic resolved structure of Sr$_{2}$IrO$_{4}$ surface in real space by using scanning tunneling microscopy. Tunneling spectroscopic results illustrate the gap opening of Sr$_{2}$IrO$_{4}$ at low temperatures with the gap size of 250 mV, indicating the metal to insulator transition. More importantly, the pair of peaks around gap in spectra suggests the quasi-particle coherent excitation, implying the Slater-type insulating state. This is further confirmed by temperature dependent measurements and density functional theory calculations.

*Research was conducted at the Center for Nanophase Materials Sciences and sponsored by the Division of Scientific User Facilities, and the Materials Sciences and Engineering Division, U.S. DOE

Authors

  • Minghu Pan

    • Center for Nanophase Materials Sciences, Oak Ridge National Laboratory
    • Oak Ridge National Laboratory
  • Qing Li

    • Oak Ridge National Laboratory
  • G.-X. Cao

    • University of Tennessee, Knoxville
  • Satoshi Okamoto

    • Oak Ridge National Laboratory
  • G. Zheng

    • Oak Ridge National Laboratory
  • Wenzhi Lin

    • Oak Ridge National Laboratory
  • Brian C. Sales

    • Oak Ridge National Laboratory
  • J.Y. Yi

    • University of Tennessee, Knoxville
  • J.-Q. Yan

    • University of Tennessee, Knoxville
  • R. Arita

    • University of Tokyo
  • J. Kunes

    • Institute of Physics, Czech Republic
  • M. Imada

    • University of Tokyo
  • D. Mandrus

    • University of Tennessee, Knoxville