Cu3Nb2O8: A Multiferroic with Chiral Coupling to the Crystal Structure

ORAL

Abstract

We will present recent bulk properties, neutron powder diffraction, and non-resonant x-ray diffraction measurements on a new multiferroic material, Cu$_3$Nb$_2$O$_8$. We demonstrate than an electric polarization evolves simultaneously with a generalised helicoidal magnetic ordering. Contrary to conventional models of multiferroicity, the electric polarization was found to lie perpendicular to the common rotation plane of the magnetic moments. We present a new model applicable to a specific class of crystals; those that support a macroscopic``ferroaxial'' vector and adopt a helicoidal magnetic structure. Our new interpretation, which may explain the multiferroic properties of a number of systems reported in recent literature, is based upon the well-understood inverse Dzyaloshinskii-Moriya interaction, but requires an altogether different interpretation.

Authors

  • Roger Johnson

    • Clarendon Laboratory, Department of Physics, University of Oxford, Oxford, OX1 3PU, United Kingdom
    • Clarendon Laboratory, Department of Physics, Oxford University, UK
  • Sunil Nair

    • IISER Pune, Sai Trinity Building, Garware Circle, Sutarwadi, Pashan, Pune, Maharashtra 411021, India
  • Laurent Chapon

    • Institut Laue-Langevin, BP 156X, 38042 Grenoble, France.
  • Alessandro Bombardi

    • Diamond Light Source, Harwell Science and Innovation Campus, Didcot, OX11 0DE, United Kingdom
  • Carlo Vecchini

    • Diamond Light Source, Harwell Science and Innovation Campus, Didcot, OX11 0DE, United Kingdom
  • D. Prabhakaran

    • Clarendon Laboratory, Department of Physics, University of Oxford, Oxford, OX1 3PU, United Kingdom
  • Andrew Boothroyd

    • Clarendon Laboratory, Department of Physics, University of Oxford, Oxford, OX1 3PU, United Kingdom
  • Paolo Radaelli

    • Clarendon Laboratory, Department of Physics, University of Oxford, Oxford, OX1 3PU, United Kingdom