Measuring Coexisting Phases in La$_{0.35}$Pr$_{0.275}$Ca$_{0.375}$MnO$_3$

ORAL

Abstract

Manganite compounds in the La$_{0.625-y}$Pr$_y$Ca$_{0.375}$MnO$_3$ series are known for exhibiting phase separation over a large temperature range. We combined the x-ray photoemission electron microscopy (PEEM) and resonant elastic soft x-ray scattering (RSXS) techniques to study the interplay between the low-temperature ferromagnetic and intermediate temperature charge-ordered/antiferromagnetic phases, respectively, in La$_{0.35}$Pr$_{0.275}$Ca$_{0.375}$MnO$_3$. We found that the system is driven by glassy polarons, which are present above the curie temperature $T_C$ in many ferromagnetic metallic manganites. They stunt the growth of the ferromagnetism on cooling: we clearly observe the onset of small, strained ferromagnetic domains almost $30\,\mathrm{K}$ above the temperature where ferromagnetism fully sets in, and the ferromagnetism has a very unconventional temperature dependence even below $T_C$. This relationship could explain the need for such high magnetic fields to induce colossal magnetoresistance.

*This research and the ALS are supported by U.S. Department of Energy, Office of Basic Energy Science.

Authors

  • Mark H. Burkhardt

    • SIMES, SLAC National Accelerator Laboratory and Stanford University
  • M.A. Hossain

    • SIMES, SLAC National Accelerator Laboratory
  • S. Sarkar

    • SIMES, SLAC National Accelerator Laboratory
  • H.A. D\"{u}rr

    • SIMES, SLAC National Accelerator Laboratory
  • J. St\"{o}hr

    • SIMES, SLAC National Accelerator Laboratory
  • Y.-D. Chuang

    • Advanced Light Source, Lawrence Berkeley National Laboratory
  • A.G. Cruz Gonzalez

    • Advanced Light Source, Lawrence Berkeley National Laboratory
  • A. Doran

    • Advanced Light Source, Lawrence Berkeley National Laboratory
  • A. Scholl

    • Advanced Light Source, Lawrence Berkeley National Laboratory
  • A.T. Young

    • Advanced Light Source, Lawrence Berkeley National Laboratory
  • Y.J. Choi

    • Rutgers Center for Emergent Materials and Department of Physics \& Astronomy
  • S.-W. Cheong

    • Rutgers Center for Emergent Materials and Department of Physics \& Astronomy