THz spectroscopy of spin waves in multiferroic Ba$_2$CoGe$_2$O$_7$ in high magnetic fields
ORAL
Abstract
By applying external magnetic field the square-lattice antiferromagnet Ba$_2$CoGe$_2$O$_7$ can be transformed to a chiral form, evidenced by large optical activity when the light is in resonance with spin excitations at sub-terahertz frequencies. We found that the magnetochiral effect, the absorption difference for the light beams propagating parallel and anti-parallel to the applied magnetic field, has an exceptionally large amplitude close to 100\% and persists to fields up to 30\,T. All these features are ascribed to the magnetoelectric nature of spin excitations as they interact both with the electric and magnetic components of light. We observe a spin flop at 15\,T, that is consistent with our theoretical calculations.
*We acknowledge the support by the Estonian Ministry of Education and Research (SF0690029s09) and Estonian Science Foundation (ETF7011, ETF8170). Part of this work has been supported by EuroMagNET II under the EU contract number 228043.
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