Circular dichroism in air-suspended single-walled carbon nanotubes

ORAL

Abstract

Chiral carbon nanotubes lack inversion symmetry and are expected to show circular dichroism. We have investigated the helicity dependence of absorption in air-suspended single-walled carbon nanotubes by using photoluminescence intensity for detection. Patterned chemical vapor deposition is used to grow carbon nanotubes over trenches etched on SiO$_{2}$/Si substrates. We identified suspended carbon nanotubes by taking photoluminescence images with a home-built laser-scanning confocal microscope and characterized them by excitation spectroscopy. A quarter-wave plate is inserted in the excitation laser path, and the photoluminescence intensity is measured as a function of the angle of the wave plate. We observe differences in the luminescence intensity between left- and right-circularly polarized light.

*This work is supported by KAKENHI and the Photon Frontier Network Program of MEXT, Japan.

Authors

  • A. Yokoyama

    • The University of Tokyo
  • A. Ishii

    • The University of Tokyo
  • M. Yoshida

    • The University of Tokyo
  • T. shimada

    • The University of Tokyo
  • Y.K. Kato

    • The University of Tokyo