Coupling of Cobalt-Tetraphenylporphyrin Molecules in Copper Nitride Molecular Network

ORAL

Abstract

We have used low temperature scanning tunneling microscopy to study the interaction between individual cobalt-tetraphenylporphyrin molecules and a molecular copper nitride network. We demonstrated that the molecular Cu$_{3}$N-Cu(110) network promotes the decoupling of the porphiryn, allowing to visualize the molecular orbitals and vibronic states of the molecule, while keeping a strong coupling of the Co atom in the center of macrocycle with the substrate. The reverse behavior was observed when the molecule was sitting on the Cu(110) metallic surface. First principle calculations confirm the assembled position of the molecule on top of N atoms and the decoupling from the surface.

Authors

  • Vinicius Claudio Zoldan

    • Laborat\'orio de Filmes Finos e Superf\'icies, Universidade Federal de Santa Catarina
  • Chunlei Gao

    • Max Planck Institute of Microstructure Physics, Halle, Germany
  • Ricardo Faccio

    • Cryssmat-Lab and Centro NanoMat, Facultad de Qu\'imica, Universidad de la Rep\'ublica, Montevideo, Uruguay
  • Andre Avelino Pasa

    • Laboratorio de Filmes Finos e Superficies, Departamento de Fisica, Universidade Federal de Santa Catarina, 88.040-900 Florianopolis, SC, Brazil
    • Laborat\'orio de Filmes Finos e Superf\'icies, Universidade Federal de Santa Catarina
    • Laboratorio de Filmes finos e Superficies (LFFS), Universidade Federal de Santa catarina