Charge transfer at the interface between ferromagnetic La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ and superconducting EuBa$_{2}$Cu$_{3}$O$_{7}$ probed by STM/STS

ORAL

Abstract

La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ (LSMO) is a ferromagnetic half-metallic compound with nearly 100{\%} spin polarization at room temperature, making it an ideal candidate for applications in spintronic devices. However, this useful functionality disappears when the thickness of LSMO film grown on SrTiO$_{3 }$substrate is reduced to below 4 nm, limiting its application in nanoscale devices. Here, we show that metallic and ferromagnetic properties of ultrathin ($<$ 4nm) LSMO film can be restored by interfacing it with a superconductor EuBa$_{2}$Cu$_{3}$O$_{7- \delta }$ (EBCO). We use scanning tunneling microscopy and spectroscopy to probe the evolution of the electronic structure of LSMO film grown on EBCO as functions of LSMO layer thickness and aging of bilayer LSMO/EBCO. Our results reveal that the charge (hole) transfer at LSMO/EBCO interface is responsible for driving LSMO film (of only five-unit-cell thickness) to metallic state. The conductive behavior of aged LSMO/EBCO bilayers varies systematically with the thickness of LSMO layer, allowing us to estimate the charge-transfer depth to be 4$\sim $5 nm on the LSMO side.

Authors

  • Yinghao Liu

    • MPA-CINT and Theoretical Division(2), Los Alamos National Laboratory, NM 87545
  • Jie Xiong

    • MPA-CINT and Theoretical Division(2), Los Alamos National Laboratory, NM 87545
  • Jason Haraldsen(2)

    • MPA-CINT and Theoretical Division(2), Los Alamos National Laboratory, NM 87545
  • Li Yan

    • MPA-CINT and Theoretical Division(2), Los Alamos National Laboratory, NM 87545
  • Alexander Balatsky(2)

    • MPA-CINT and Theoretical Division(2), Los Alamos National Laboratory, NM 87545
  • Quanxi Jia

    • MPA-CINT and Theoretical Division(2), Los Alamos National Laboratory, NM 87545
  • Antoinette Taylor

    • MPA-CINT and Theoretical Division(2), Los Alamos National Laboratory, NM 87545
  • Dmitry Yarotski

    • MPA-CINT and Theoretical Division(2), Los Alamos National Laboratory, NM 87545