Lattice-Symmetry-Driven Phase Competition in Vanadium Dioxide

POSTER

Abstract

We performed group-theoretical analysis of the symmetry relationships between lattice structures of R, M1, M2, and T phases of vanadium dioxide in the frameworks of the general Ginzburg-Landau phase transition theory. The analysis leads to a conclusion that the competition between the lower-symmetry phases M1, M2, and T in the metal-insulator transition is pure symmetry driven, since all the three phases correspond to different directions of the same multi-component structural order parameter. Therefore, the lower-symmetry phases can be stabilized in respect to each other by small perturbations such as doping or stress.

*Work at ORNL's CNMS was sponsored by DSUF OBES, U.S. DOE. Work at SIUC was funded through NSF 772 ECCS-0925837 and SISGR-DOE ERKCM67. J.D.B. and J.Z.T. were supported by MSED OBES, U.S. DOE. IL was supported by ANR project LOMACOQU.

Authors

  • Alexander Tselev

    • Oak Ridge National Laboratory, Oak Ridge, TN, USA
    • Oak Ridge National Laboratory, Oak Ridge, TN
  • Igor A. Luk'yanchuk

    • University of Picardie Jules Verne, Amiens, France
  • Ilia N. Ivanov

    • Oak Ridge National Laboratory, Oak Ridge, TN, USA
  • John D. Budai

    • Oak Ridge National Laboratory, Oak Ridge, TN, USA
  • Jonathan Z. Tischler

    • Oak Ridge National Laboratory, Oak Ridge, TN, USA
  • Evgheni Strelcov

    • Southern Illinois University Carbondale, Carbondale, IL, USA
  • Andrei Kolmakov

    • Southern Illinois University Carbondale, Carbondale, IL, USA
  • Sergei V. Kalinin

    • Oak Ridge National Laboratory, Oak Ridge, TN, USA