Broken vector spin chirality in biatomic Fe chains on Ir(001)

ORAL

Abstract

We investigate from {\em ab initio} the magnetism of biatomic Fe chains, which form due to self-organization on the (5$\times$1)-reconstructed Ir(001) surface [1,2]. Using the {\tt FLEUR} code [3], we calculate the magnetic properties and exchange interactions in this system, finding a very small Heisenberg exchange along the chain of the order of 10 meV/Fe-atom. Upon including spin-orbit coupling we obtain the contribution from the Dzyaloshinskii-Moriya interaction and find that it leads to a 120$^{\circ}$ spin-spiral ground state of the Fe chains with a unique rotational sense. The results of the Monte-Carlo simulations based on the parameters from {\it ab initio} are in a very good agreement to STM experiments on the system. Moreover, simulations indicate a robustness of the spin chiral order parameter, which decays with temperature much slower than the scalar spin correlation, in analogy to a vector spin chiral liquid state. We discuss possible applications of the magnetism in these chains with respect to the transfer of information on the nanoscale.\newline [1] L. Hammer {\it et al.}, Phys. Rev. B {\bf 67}, 125422 (2003). [2] Y. Mokrousov \textit{et al.}, Phys. Rev. B \textbf{80}, 195420 (2009). [3] www.flapw.de

*We acknowledge funding under HGF-YIG Programme VH-NG-513.

Authors

  • Stefan Bl\"ugel

    • Institute for Advanced Simulation, Research Centre Juelich, Germany
    • Peter Gr\"unberg Institut and Institute for Advanced Simulation, Forschungszentrum J\"ulich and JARA, 52425 J\"ulich, Germany
    • Peter Grunberg Institut and Institute for Advanced Simulation, Forschungszentrum Juelich and JARA, 52425 Juelich, Germany
    • Peter Gr\"unberg Institut (PGI) and Institute for Advanced Simulation (IAS), Forschungszentrum J\"ulich and JARA, 52425-J\"ulich, Germany
    • Peter Gruenberg Institut (PGI-1) \& Institute for Advanced Simulation (IAS-1), Forschungszentrum Juelich and JARA, 52425 Juelich, Germany
    • Forschungszentrum Juelich, Germany
  • Y. Mokrousov

    • Peter Grunberg Institut and Institute for Advanced Simulation, Forschungszentrum Juelich and JARA, 52425 Juelich, Germany
  • M. Menzel

    • Institut fur Angewandte Physik, Universitat Hamburg, 20355 Hamburg, Germany
  • R. Wieser

    • Institut fur Angewandte Physik, Universitat Hamburg, 20355 Hamburg, Germany
  • K. von Bergmann

    • Institut fur Angewandte Physik, Universitat Hamburg, 20355 Hamburg, Germany
  • E. Vedmedenko

    • Institut fur Angewandte Physik, Universitat Hamburg, 20355 Hamburg, Germany
  • A. Kubetzka

    • Institut fur Angewandte Physik, Universitat Hamburg, 20355 Hamburg, Germany
  • R. Wiesendanger

    • Institut fur Angewandte Physik, Universitat Hamburg, 20355 Hamburg, Germany
  • S. Heinze

    • Institut fur Theoretische Physik und Astrophysik, Christian-Albrecht-Universitat zu Kiel, 24098 Kiel, Germany