Composition spread studies of (RE)NiO$_{3}$-LaNiO$_{3}$ thin films

ORAL

Abstract

Epitaxial thin films of La$_{x}$Nd$_{1-x}$NiO$_{3}$ and La$_{x}$Pr$_{1-x}$NiO$_{3}$ were grown via pulsed laser deposition on SrTiO$_{3}$ (001) with an automated~moving shutter system to create 100 nm thick composition spreads. These films have the advantage of providing a continuous spectrum of doping compositions at the same deposition conditions, such as temperature and oxygen pressure, without the need to prepare different stoichiometric targets or perform different depositions for desired compositions.~Composition evolution is verified via wavelength dispersive spectroscopy, and x-ray diffraction mapping shows that the lattice constant of the film varies continuously from LaNiO$_{3}$ to NdNiO$_{3}$. Simultaneous measurements of resistance versus temperature down to 4.2 K across the spreads show evolution in transport behavior. The details will be discussed.

*Funding provided by AFO SR MURI Grant \#FA95500910603 and NSF MRSEC @ UMD (DMR 0520471).

Authors

  • Richard Suchoski

    • University of Maryland, College Park - MSE, CNAM
  • I. Takeuchi

    • Department of Materials Science and Engineering, University of Maryland, College Park, MD 20424
    • University of Maryland, College Park - MSE, CNAM
    • Deparment of Materials Science and Engineering, University of Maryland, College Park, MD 20424
  • Kui Jin

    • University of Maryland
    • Center for Nanophysics \& Advanced Materials, Department of Physics, University of Maryland, College Park
    • University of Maryland, College Park - Physics, CNAM
  • Richard Greene

    • University of Maryland, College Park - Physics, CNAM