Giant Bipolar Nernst Effect in the Quasi-One-Dimensional Metal, Li$_{0.9}$Mo$_6$O$_{17}$

ORAL

Abstract

The Nernst coefficient for the quasi-one-dimensional metal, Li$_{0.9}$Mo$_6$O$_{17}$, is found to be among the largest known for metals ($\nu\simeq 500\ \mu$V/KT at $T\sim 20$~K), and is enhanced in a broad range of temperature by orders of magnitude over the value expected from Boltzmann theory for carrier diffusion. A comparatively small Seebeck coefficient implies that Li$_{0.9}$Mo$_6$O$_{17}$ is bipolar with large, partial Seebeck coefficients of opposite sign. A very large thermomagnetic figure of merit, $ZT\sim 0.5$, is found at high field in the range $T\approx 35-50$~K.

*This material is based upon work supported by an award from Research Corporation (Univ.~Miami), the National Science Foundation under grant DMR-0907036 (Mont.~St.~Univ.), and in Lorena by the CNPq (301334/2007-2) and FAPESP (2009/14524-6).

Authors

  • Joshua L. Cohn

    • University of Miami
  • Benjamin D. White

    • Department of Physics, University of California, San Diego, La Jolla, CA 92093, USA
    • University of California, San Diego
    • Montana State University
  • Carlos A. M. dos Santos

    • Escola de Engenharia de Lorena - USP, Brazil
  • John J. Neumeier

    • Montana State University