Probing the timescale of the exchange interaction in a ferromagnetic alloy

ORAL

Abstract

The underlying physics of all ferromagnetic behavior is the cooperative interaction between individual atomic magnetic moments that results in a macroscopic magnetization. In this work, we use extreme ultraviolet pulses from high-harmonic generation as an element-specific probe of ultrafast, optically driven, demagnetization in a ferromagnetic Fe-Ni alloy (Permalloy). We show that for times shorter than the characteristic timescale for exchange coupling, the magnetization of Fe quenches more strongly than that of Ni. Then, as the Fe moments start to randomize, the strong ferromagnetic exchange interaction induces further demagnetization in Ni, with a characteristic delay determined by the strength of the exchange interaction. We can further enhance this delay by lowering the exchange energy by diluting the Permalloy with Cu. This measurement probes how the fundamental quantum mechanical exchange coupling between Fe and Ni in magnetic materials influences magnetic switching dynamics in ferromagnetic materials relevant to next-generation data storage technologies.

Authors

  • Emrah Turgut

    • JILA, University of Colorado, Boulder
  • Chan La-O-Vorakiat

    • JILA, University of Colorado, Boulder
  • Mark E. Siemens

    • JILA, University of Colorado, Boulder
  • Margaret M. Murnane

    • JILA, University of Colorado, Boulder
  • Henry C. Kapteyn

    • JILA, University of Colorado, Boulder
  • Stefan Mathias

    • University of Kaiserslautern and Research Center OPTIMAS, Germany
  • Patrick Granitzka

    • University of Kaiserslautern and Research Center OPTIMAS, Germany
  • Steffen Eich

    • University of Kaiserslautern and Research Center OPTIMAS, Germany
  • Martin Aeschlimann

    • University of Kaiserslautern and Research Center OPTIMAS, Germany
  • Patrik Grychtol

    • Peter Gr\"unberg Institute, Research Center J\"ulich, Germany
  • Roman Adam

    • Peter Gr\"unberg Institute, Research Center J\"ulich, Germany
  • Claus M. Schneider

    • Peter Gr\"unberg Institute, Research Center J\"ulich, Germany
  • Justin M. Shaw

    • National Institute of Standards and Technology, Boulder
  • Hans T. Nembach

    • National Institute of Standards and Technology, Boulder
  • Thomas J. Silva

    • National Institute of Standards and Technology, Boulder