Nonequilibrium ``melting'' of a charge density wave insulator via an ultrafast infrared laser pulse

ORAL

Abstract

In equilibrium, electrons interacting with lattice vibrations have a transition either to a charge density wave phase (a static modulation of the electronic charge) or to a superconductor (electron pairs move without resistance). If the coupling is weak, the system orders in the Bardeen-Cooper-Schrieffer scenario, where the ordering occurs at some transition temperature Tc and a gap simultaneously forms in the density of states. In strong-coupling, preformed pairs bind at a high temperature (forming a gap in the density of states) and the ordering only occurs at a lower temperature. We employ an exact solution of a model for pump-probe time-resolved photoemission spectroscopy to show how, in nonequilibrium, a third scenario arises: the gap disappears in the presence of a nonzero order parameter, and then reforms well after the pulse has passed. This nonequilibrium ``phase transition'' scenario qualitatively describes all of the available experiments on the ultrafast melting of a charge density wave.

*National Science Foundation, Department of Energy, National Energy Research Scientific Computing Center

Authors

  • Wen Shen

    • Georgetown University
  • Yizhi Ge

    • Georgetown University
  • Amy Liu

    • Georgetown University
    • Physics Department, Georgetown University
  • H.R. Krishnamurthy

    • Center for Condensed Matter Theory, Indian Institute of Science, Bangalore 560012, India
    • Department of Physics, Indian Institute of Science, Bangalore 560012, India
    • India Institute of Science
  • Tom Devereaux

    • Department of Physics, Stanford University, Stanford
    • SIMES, SLAC National Accelerator Laboratory and Stanford University
    • Stanford Institute for Materials and Energy Science
    • Stanford Institute for Materials and Energy Science, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025, USA
    • Stanford Institute for Materials and Energy Science, SLAC National Accelerator Laboratory
    • Stanford University and SLAC National Accelerator Laboratory
    • Stanford University
  • Jim Freericks

    • Georgetown University