Magnetic ordering in EuCo$_2$As$_2$

ORAL

Abstract

We have synthesized and studied EuCo$_2$As$_2$ single crystals by resistivity, magnetoresistance, and susceptibility measurements. We found antiferromagnetic (AFM) ordering of the Eu spins at $T_N = 50$ K. Upon applying a magnetic field $H \| ab$ at $T = 2$ K this phase exhibits a metamagnetic (MM) transition at $H_{MM} = 3.5$ T. In case of $H \| c$ the magnetisation increases linearly up to 7 T. The same AFM to MM transition was found at 0.5 T in EuFe$_2$As$_2$ where it was found to be due to the reorientation of the Eu spin. We found that replacing Fe with Co strengthens the coupling between the Eu moments resulting in a higher $T_N$ and H$_{MM}$.

*Research sponsored by the Material Science and Engineering Division Office of Basic Energy Sciences, U. S. Department of Energy.

Authors

  • Balazs Sipos

  • A.S. Sefat

    • ORNL
    • Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
    • Oak Ridge National Laboratory
    • MST Division, Oak Ridge National Laboratory
    • ORNL, Oak Ridge, TN
    • Oak Ridge National Laboratory (ORNL), Oak Ridge, TN 37831, USA
    • Materials Science \& Technology Division, ORNL, Oak Ridge, TN 37831, USA
  • B.C. Sales

    • ORNL
    • Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
    • Oak Ridge National Laboratory
    • Oak Ridge National Laboratory (ORNL), Oak Ridge, TN 37831, USA
    • Materials Science \& Technology Division, ORNL, Oak Ridge, TN 37831, USA