Spontaneous Vortex Nanodomain Arrays at Ferroelectric Heterointerfaces

ORAL

Abstract

The polarization of BiFeO$_{3}$ subjected to different electrical boundary conditions by hetero-interfaces is imaged with atomic resolution using a Cs-corrected transmission electron microscope. Unusual nanodomains are seen and their role in providing polarization closure is understood through phase-field simulations. Hetero-interfaces are key to the performance of ferroelectric devices and this first observation of vortex arrays at ferroelectric hetero-interfaces reveals properties unlike the surrounding film including mixed Ising-N\'{e}el domain walls, which will affect switching behavior, and a drastic increase of in-plane polarization. Imaging this magnetic analogous effect at ferroelectric hetero-interfaces provides the ability to see device-relevant interface issues.

Authors

  • Xiaoqing Pan

    • Dept. of Mater. Sci. \& Eng., Univ. of Michigan, Ann Arbor, MI
    • Department of Materials Science and Engineering, University of Michigan, Ann Arbor, MI 48109
    • University of Michigan
  • Christopher Nelson

    • Dept. of Mater. Sci. \& Eng., Univ. of Michigan, Ann Arbor, MI
  • Yi Zhang

    • Dept. of Mater. Sci. \& Eng., Univ. of Michigan, Ann Arbor, MI
  • Benjamin Winchester

    • Dept. of Mater. Sci. \& Eng., Penn State Univ., University Park, PA
  • Long-Qing Chen

    • Dept. of Mater. Sci. \& Eng., Penn State Univ., University Park, PA
  • Colin Heikes

    • Dept. Sci. \& Eng., Cornell Univ., Ithaca, NY
  • Carolina Adamo

    • Dept. Sci. \& Eng., Cornell Univ., Ithaca, NY
  • Alexander Melville

    • Dept. Sci. \& Eng., Cornell Univ., Ithaca, NY
  • Darrell Schlom

    • Dept. Sci. \& Eng., Cornell Univ., Ithaca, NY
  • Chad Folkman

    • Dept. of Mater. Sci. \& Eng., Univ. of Wisconsin-Madison, Madison, WI
  • Chang-Beom Eom

    • Dept. of Mater. Sci. \& Eng., Univ. of Wisconsin-Madison, Madison, WI