Low-Frequency Vibrational Modes and Rearrangements in a Colloidal Glass Subject to Point Expansion

ORAL

Abstract

We conduct experiments on two-dimensional packings of colloidal thermosensitive hydrogel particles. The packing fraction of the colloidal suspension is tunable from liquid to deeply jammed by varying the global temperature of the sample. In addition, by tightly focusing an infrared laser on the sample, point expansion of the colloidal glass is induced via thermophoretic forces. We utilize displacement correlation matrix techniques employed in recent papers, and we employ video microscopy to derive the vibrational modes. The response of the sample to induced point expansion is analyzed over a range of packing fractions, with particular focus on the correlation between quasi-localized low-frequency vibrational modes and regions of rearrangements.

*This research is supported by an award from Research Corporation (KBA), MRSEC grant DMR-0520020 (AGY), NSF grant DMR-0804881 (AGY), and NASA grant NNX08AO0G (AGY).

Authors

  • Kevin Aptowicz

    • West Chester University
  • Matthew Colagreco

    • West Chester University
  • Ryan Margolis

    • West Chester University
  • Peter Yunker

    • University of Pennsylvania
    • Department of Physics and Astronomy, University of Pennsylvania
  • Ke Chen

    • University of Pennsylvania
    • Department of Physics and Astronomy, University of Pennsylvania
  • Arjun Yodh

    • Physics and Astronomy, University of Pennsylvania
    • University of Pennsylvania
    • Department of Physics and Astronomy, University of Pennsylvania