Formation of collapsed tetragonal phase in EuCo$_{2}$As$_{2}$ under high pressure

ORAL

Abstract

The structural properties of EuCo$_{2}$As$_{2}$ have been studied up to 35 GPa, through the use of x-ray diffraction in a diamond anvil cell at a synchrotron source. At ambient conditions, EuCo$_{2}$As$_{2}$ ($I$4/\textit{mmm}) has a tetragonal lattice structure with a bulk modulus of 48 $\pm $ 4 GPa. With the application of pressure, the $a $axis exhibits negative compressibility with a concurrent sharp decrease in $c$-axis length. The anomalous compressibility of the $a $axis continues until 4.7 GPa, at which point the structure undergoes a second-order phase transition to a collapsed tetragonal (CT) state with a bulk modulus of 111 $\pm $ 2 GPa. We found a strong correlation between the ambient pressure volume of 122 parents of superconductors and the corresponding tetragonal to collapsed tetragonal phase transition pressures.

*MB acknowledges support from the National Science Foundation (NSF) Research Experiences for Undergraduates (REU)-site under grant no. NSF-DMR-06446842.

Authors

  • Matthew Bishop

    • University of West Georgia (UWG), Carrollton, GA 30118, USA
  • Walter Uhoya

    • University of Alabama at Birmingham (UAB), Birmingham, AL 35294, USA
  • Georgiy Tsoi

    • University of Alabama at Birmingham (UAB), Birmingham, AL 35294, USA
    • University of Alabama at Birmingham
  • Yogesh Vohra

    • Department of Physics, University of Alabama at Birmingham
    • University of Alabama at Birmingham (UAB), Birmingham, AL 35294, USA
    • University of Alabama at Birmingham
  • A.S. Sefat

    • ORNL
    • Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
    • Oak Ridge National Laboratory
    • MST Division, Oak Ridge National Laboratory
    • ORNL, Oak Ridge, TN
    • Oak Ridge National Laboratory (ORNL), Oak Ridge, TN 37831, USA
    • Materials Science \& Technology Division, ORNL, Oak Ridge, TN 37831, USA
  • B.C. Sales

    • ORNL
    • Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
    • Oak Ridge National Laboratory
    • Oak Ridge National Laboratory (ORNL), Oak Ridge, TN 37831, USA
    • Materials Science \& Technology Division, ORNL, Oak Ridge, TN 37831, USA