Spin dynamics in the hyperkagome compound Gd$_{3}$Ga$_{5}$O$_{12}$
COFFEE_KLATCH · Invited
Abstract
We present the first neutron inelastic scattering results on the magnetic state of the frustrated hyperkagome compound $\rm Gd_3Ga_5O_{12}$ (GGG) at low temperatures and in applied magnetic field. Our neutron scattering studies reveal a remarkable range of timescales. Short-range spatial correlations appear static within the instrumental resolution (50~$\mu$eV). Three distinct inelastic modes are found at 0.04(1), 0.12(2) an 0.58(3)~meV at 0.06~K. The application of a magnetic field up to 2.5~tesla reveals disparate behavior of the magnetic excitations. In zero applied field, the lowest and highest energy excitations show spatial dependencies indicative of dimerized short-range antiferromagnetic correlations that survive to high temperatures, comparable to the nearest neighbor exchange interactions. Our results suggest that the ground state of a three dimensional hyperkagome compound differs distinctly from its frustrated counterparts on a pyrochlore lattice and reveal a juxtaposition of cooperative paramagnetism and strong dimerized coupling. These results are surprising since GGG is often classified as a strongly frustrated system with a manifold of connected states for which one would expect a continuum of gapless excitations. \\[4pt] In collaboration with: Pascale Deen, Institut Laue Langevin; G. Balakrishnan, Department of Physics, University of Warwick; B.D. Rainford, Department of Physics and Astronomy, Southampton University; C. Ritter, Institut Laue-Langevin; L. Capogna, Istituto Officina dei Materiali, IOM-CNR; H. Mutka and T. Fennell, Institut Laue-Langevin.
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