Many-body large polaron optical conductivity in SrTi$_{1-x}$Nb$_{x}$O$_{3}$

ORAL

Abstract

Recent experimental data on the optical conductivity of niobium doped SrTiO$_{3}$ are interpreted in terms of a gas of large polarons. The theoretical approach takes into account many-body effects, the electron-phonon interaction with multiple LO-phonon branches, and the degeneracy and the anisotropy of the Ti t$_{2g}$ conduction band. The many-body large-polaron model based on the Fr\"{o}hlich interaction provides a fair agreement between the theoretical large-polaron optical conductivity band and the experimental mid-infrared optical conductivity band without any adjustment of material parameters. The large-polaron model gives then a convincing interpretation of the experimentally observed optical conductivity spectra of SrTi$_{1-x}$Nb$_{x}$O$_{3}$.

*This work was supported by FWO-V projects G.0356.06, G.0370.09N, G.0180.09N, G.0365.08, the WOG WO.035.04N (Belgium), and by the Swiss National Science Foundation under Grant No. 200020-125248 and NCCR Materials with Novel Electronic Properties--MaNEP.

Authors

  • J.T. Devreese

    • Theorie van Quantum en Complexe Systemen, Universiteit Antwerpen, Antwerpen, Belgium
    • Universiteit Antwerpen
  • S. N. Klimin

    • Theorie van Quantum en Complexe Systemen, Universiteit Antwerpen, Antwerpen, Belgium
  • J. L. M. van Mechelen

    • Departement de Physique de la Mati\`{e}re Condensee, Universite de Gen\`{e}ve, Gen\`{e}ve, Switzerland
  • D. van der Marel

    • Departement de Physique de la Mati\`{e}re Condensee, Universite de Gen\`{e}ve, Gen\`{e}ve, Switzerland