Neutron Diffraction Studies of Structural and Magnetic Phase Transitions in Ru Doped [1111] Fe Pnictides

ORAL

Abstract

We report neutron diffraction studies of pnictide [1111] compounds PrFe(1-x)Ru(x)AsO. The undoped parent compound PrFeAsO undergo transitions from a tetragonal to an orthorhombic crystal structure, as well as transitions to a state of magnetic order. Doping on different sites can induce various ground states, including superconductivity. Here we examine the effect of substitutionally doping Ru for Fe. In particular we report neutron diffraction measurements for PrFe (1-x)Ru(x)AsO with x=0, 0.33 and 0.75. Previous bulk and x-ray measurements (M. A. McGuire et al., J. Sol. St. Chem. 182, 2326 (2009)) have shown that doping with Ru moves the structural transition to lower temperature and can also suppress the magnetic order. The neutron diffraction confirms this and shows no sign of magnetic order down to 4K for x=0.33 or 0.75.

*Supported by US DOE BES Science Facilities and Materials Research

Authors

  • Yuen Yiu

    • University of Tennessee- Physics
  • Vasile Garlea

    • Oak Ridge National Laboratory - NSSD
  • Stephen Nagler

    • Oak Ridge National Laboratory
    • Oak Ridge National Laboratory - NSSD
  • Michael McGuire

    • Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831
    • Oak Ridge National Laboratory, Oak Ridge, Tennessee
    • Oak Ridge National Laboratory - MSTD
    • Oak Ridge National Laboratory
  • Brian Sales

    • Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831
    • ORNL
    • Oak Ridge National Laboratory, Oak Ridge, Tennessee
    • Oak Ridge National Laboratory
    • Oak Ridge National Laboratory - MSTD
  • Athena Sefat

  • David Mandrus

    • Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831
    • ORNL
    • Oak Ridge National Laboratory, Oak Ridge, Tennessee
    • Oak Ridge National Laboratory - MSTD
    • Oak Ridge National Laboratory