Oxygen-isotope-substitution-induced nanoscale crystallinity and origin of metal-insulator transition in Sm$_{0.5}$Sr$_{0.5}$MnO$_{3}$
ORAL
Abstract
Competing effects of $^{16}$O$\rightarrow^{18}$O isotope substitution and magnetic field on the phase separation and structural property in Sm$_{0.5}$Sr$_{0.5}$MnO$_{3}$ have been studied by using high-resolution high-energy X-ray diffraction under magnetic fields up to 7 T. A close correlation between physical properties and the crystallinity of the compounds is observed. The oxygen-isotope-substitution-induced metal-insulator transition is caused by nanoscale crystallite formation in the compound with $^{18}$O below a phase-separation temperature T$_{ps} \sim 100$ K. Different lattice effects on the magnetoresistance are identified, among which the largest one is due to magnetic field enhanced crystallization of the nanoscale crystallites.
*Use of the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357.
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