Spin Correlation and Magnetically Induced Ferroelectricity in YMn$_2$O$_5$

ORAL

Abstract

There is great interest in understanding the microscopic nature of the coupling between ferroelectricity and magnetic ordering in several multiferroic frustrated manganites $R$MnO$_3$ and $R$Mn$_2$O$_5$ ($R$= rare earth and Y). For $R$MnO$_3$, the multiferroicity can be understood in terms of the anti- symmetric spin interaction, whereas the underlying mechanism of multiferroicity in $R$Mn$_2$O$_5$ remains controversial, because of its structural complexity. We unraveled the temperature-dependent spin ordering of multiferroic YMn$_2$O$_5 $ by using resonant soft x-ray magnetic scattering at Mn $L_3$ edge. For temperatures below the onset temperature $T_C$ of ferroelectricity, the handedness of cycloidal spin spirals exists, but vanishes above $T_C$. The spin handedness perpendicular to the induced polarization reverses at the temperature where the polarization changes its sign. The temperature dependence of spin correlation along the propagating direction of spin spirals resembles the temperature behavior of polarization. These data imply that both symmetric and antisymmetric spin interactions involve in the magnetoelectric coupling in YMn$_2$O$_5$.

Authors

  • J. Okamoto

    • National Synchrotron Radiation Research Center, Taiwan
  • D. J. Huang

    • National Synchrotron Radiation Research Center, Taiwan
  • W. B. Wu

    • National Synchrotron Radiation Research Center, Taiwan
  • S. L. Cheng

    • National Synchrotron Radiation Research Center, Taiwan
  • C. T. Chen

    • National Synchrotron Radiation Research Center, Taiwan
  • C. Y. Mou

    • National Center for Theoretical Sciences, Taiwan
  • K. S. Chao

    • National Chiao-Tung University, Taiwan
  • S. W. Huang

    • National Chiao-Tung University, Taiwan
  • S. Park

    • Rutgers University, USA
  • S-W. Cheong

    • Rutgers University, USA