Temperature-dependent electronic structure evolution of spin-orbit coupling induced Mott insulator Sr$_{2}$IrO$_{4}$

ORAL

Abstract

Recently, the effect of spin-orbit coupling in 5$d$ transition metal oxides attracted lots of attention. It was found that the cooperative interaction of spin-orbit coupling and electron correlation could realize unique Mott insulating ground state of Sr$_{2}$IrO$_{4}$. We investigated temperature-dependent optical conductivity spectra of 5$d$ Mott insulator Sr$_{2}$IrO$_{4}$. We observed drastic changes of the optical conductivity spectra. As temperature increases, the Mott gap was significantly reduced and spectral weight redistribution between the Ir $t_{2g}$ bands occurred. The electronic structure changes accompanied the change of optical phonon modes. These experimental observations could be understood in terms of the effects of spin-orbit and electron-lattice coupling.

Authors

  • S. J. Moon

  • W. S. Choi

  • T. W. Noh

    • ReCOE and FPRD, Department of Physics and Astronomy, Seoul National University, Seoul 151-747, Korea
  • H. Jin

    • CSCMR, Department of Physics and Astronomy, Seoul National University, Seoul 151-747, Korea
  • Y. S. Lee

    • Department of Physics, Soongsil University, Seoul 156-743, Korea
  • G. Cao

    • Department of Physics and Astronomy, University of Kentucky, Lexington, Kentucky 40506, USA