Enhanced ferroelectric polarization by induced Dy spin-order in multiferroic DyMnO$_{3}$

ORAL

Abstract

Neutron powder diffraction and single crystal x-ray resonant magnetic scattering measurements suggest that Dy plays an active role in enhancing the ferroelectric polarization in multiferroic DyMnO$_{3}$ above $T_{N}^{\rm Dy}$=~6.5~K. We observe the evolution of an incommensurate ordering of Dy moments with the same periodicity as the Mn spiral ordering. It closely tracks the evolution of the ferroelectric polarization. Below $T_{N}^{\rm Dy}$, where Dy spins order commensurately, the polarization decreases to values similar for those of TbMnO$_{3}$. The higher $P_{s}$~found just above $T_{N}^{\rm Dy}$~arises from the contribution of Dy-spins so as to effectively increase the amplitude of the Mn spin-spiral.

Authors

  • O. Prokhnenko

  • R. Feyerherm

  • E. Dudzik

  • S. Landsgesell

  • N. Aliouane

    • Hahn-Meitner-Institut, Glienicker Str. 100, Berlin D-14109, Germany
  • L.C. Chapon

    • ISIS, Rutherford Appleton Laboratory, Chilton, Didcot, OX11, 0QX United Kingdom
  • D.N. Argyriou

    • Hahn-Meitner-Institut, 100 Glienicker str, Berlin, Germany
    • HMI
    • Hahn-Meitner-Institut, Glienicker Str. 100, Berlin D-14109, Germany
    • Hahn-Meitner-Institut
    • HMI, Berlin, Germany