Observation of coherent high-wavevector acoustic vibrations in a bulk material using time-resolved X-ray diffraction

ORAL

Abstract

We report on the observation of high-wavevector acoustic phonons in bulk InP that originate from folded phonons in a GaInAs/AlInAs superlattice. Synchrotron time-resolved X-ray diffraction is used to probe the evolution of the laser-generated acoustic phonons. Due to the short wavelength, X-ray diffraction gives access high-wavevector components of the acoustic wave-packet in a bulk material. Experiments show a bulk excitation at a wavevector $q=2 \pi/D$, where $D$ is the superlattice period, which propagates into the substrate at the speed of sound. These results are supported by time-resolved dynamical diffraction calculations in which the strain is included as a perturbation from the perfect crystal.

*This work was conducted at the sector 7 insertion device beamline at the APS and was supported in part by the U.S. DoE and from the NSF FOCUS physics frontier center.

Authors

  • Mariano Trigo

    • University of Michigan
  • Yu-Miin Sheu

    • University of Michigan
  • Emily Peterson

    • University of Michigan
  • David Reis

    • University of Michigan
  • Matthew Reason

    • University of Michigan
  • Rachel Goldman

    • University of Michigan
  • Roberto Merlin

    • University of Michigan
  • Eric Landahl

    • Argonne National Laboratory
  • Donald Walko

  • Dohn Arms

    • Argonne National Laboratory