Discontinuity of the dielectric function at Bragg reflexes

POSTER

Abstract

As an example for layered materials, the loss function of graphite was studied for momentum transfers $q$ beyond the first Brillouin zone. Surprisingly, near Bragg reflexes, the spectra are highly dependent on very small changes in $q$, which reminds the non-analyticity of the loss function in the optical limit ($q\!\to\!0$). The effect is investigated by means of first principle calculations within the random phase approximation (RPA) and is confirmed by inelastic x-ray spectroscopy (IXS) measurements. We find crystal local field effects to be crucial and propose a simple $2\!\times\! 2$ model dielectric function for explanation.

Authors

  • R. Hambach

    • LSI, CEA-CNRS UMR 7642-Ecole Polytechnique, France and ETSF France
  • C. Giorgetti

    • LSI, CEA-CNRS UMR 7642-Ecole Polytechnique, France and ETSF France
  • F. Sottile

    • LSI, CEA-CNRS UMR 7642-Ecole Polytechnique, France and ETSF France
  • L. Reining

    • LSI, CEA-CNRS UMR 7642-Ecole Polytechnique, France and ETSF France
  • N. Hiraoka

    • National Synchrotron Radiation Research Center , Hsinchu 30076 , Taiwan
  • Y.Q. Cai

    • National Synchrotron Radiation Research Center , Hsinchu 30076 , Taiwan
  • A.G. Marinopoulos

    • Department of Physics and Astronomy, Vanderbilt University, Nashville, USA
  • F. Bechstedt

    • IFTO, Friedrich-Schiller Universitaet Jena, Germany