Field Effect on Spin Correlations in La$_{1-x}$Sr$_x$CoO$_3$

ORAL

Abstract

La$_{1-x}$Sr$_x$CoO$_3$ evolves from a non-magnetic, insulating ground state in the parent compound (x=0) into a metallic, ferromagnetic cluster-glass (x$>$0.18). For intermediate concentrations, the ground state is characterized by a competition between ferromagnetic and incommensurate spin correlations, which leads to short-range clustering. The field effect on these competing spin correlations has been investigated by neutron diffraction from a single crystal of La$_{.85}$Sr$_{.15}$CoO$_3$ under an externally applied vertical magnetic field ranging from 0 to 7 T. The intensity of the incommensurate reflections is signficantly reduced under 7 T. On the other hand, the ferromagnetic signal is enhanced by more than an order of magnitude under 7 T, while simultaneously narrowing in reciprocal space, implying an increase in the correlation length, which cannot be understood simply by a reorientation of ferromagnetic clusters along the direction of the applied field. Instead, the data is interpreted in a phase-separated scenario in which the applied field polarizes regions which are initially not ferromagnetic in zero field.

Authors

  • Daniel Phelan

    • National Institute of Standards and Technology
  • Despina Louca

    • University of Virginia
  • Seunghun Lee

    • University of Virginia
  • Stine Ancona

    • Argonne National Laboratory
  • Stephan Rosenkranz

    • Argonne National Laboratory
  • John Mitchell

    • Argonne National Laboratory