Non-classical scaling in the Pb/Si(111) coarsening at low temperature

ORAL

Abstract

Recent coarsening experiments monitoring the evolution of a mixture of stable and unstable islands in Pb/Si(111) towards a mono-disperse 7-layer height distribution have revealed novel features that extend the classical curvature driven growth. Two complementary techniques are used, X-ray scattering and STM. In particular the coverage $\theta $ , temperature T and flux F dependence are the opposite of what is expected from the classical analysis. The coarsening time $\tau $ increases with increasing temperature T, coverage $\theta $ and decreases with increasing flux rate F according to the scaling relation $\tau $F=constant. These paradoxical results can be understood from the island stability dependence on lateral size L in addition to the QSE-driven well--analyzed height dependence. The decay constant of an unstable island is an increasing function of its lateral size and for sizes larger than Lc$\sim $50nm the unstable islands do not decay but grow in the next stable height. Since the lateral size increases with T, $\theta $ and decreases with F this can account for the novel coarsening results.

*Acknowledgement: NSF(DMR0706278), PRF(41792-AC10), Advanced Photon Source(DOE), Ames Lab is supported by Department of Energy-Basic Sciences under Contract DE-AC02-07CH11358.

Authors

  • M. Hupalo

    • Iowa State University Ames Lab-USDOE
    • Iowa State University and Ames Laboratory of US-DOE
  • R. Feng

    • MUCAT, Advanced Photon Source, Argonne National Laboratory
  • E.H. Conrad

    • MUCAT, Advanced Photon Source, Argonne National Laboratory
  • C. A. Jeffrey

    • MUCAT, Advanced Photon Source, Argonne National Laboratory
  • P. F. Miceli

    • MUCAT, Advanced Photon Source, Argonne National Laboratory
  • S. Hayden

    • MUCAT, Advanced Photon Source, Argonne National Laboratory
  • M. Gramlich

    • MUCAT, Advanced Photon Source, Argonne National Laboratory
  • P. J. Ryan

    • MUCAT, Advanced Photon Source, Argonne National Laboratory
  • C. Kim

    • MUCAT, Advanced Photon Source, Argonne National Laboratory
  • M.C. Tringides

    • Iowa State University Ames Lab-USDOE