High-Energy Magneto-Dielectric Effect in Co$_{3}$V$_{2}$O$_{8}$.

ORAL

Abstract

We investigate the optical and magneto-optical properties of the Kagom\'{e} staircase compound Co$_{3}$V$_{2}$O$_{8}$ in order to explore mechanistic aspects of the high-energy magneto-dielectric effect. Co$_{3}$V$_{2}$O$_{8}$ displays a much smaller dielectric contrast compared to quasi-isostructural Ni$_{3}$V$_{2}$O$_{8}$, a result that we attribute to a high-temperature local structural distortion in Co$_{3}$V$_{2}$O$_{8}$ along the cross-tie direction. Such a distortion prevents the low temperature magnetic transitions from having a strongly coupled lattice component. This proposition is supported by vibrational studies.

*This work is supported by the U.S. Department of Energy.

Authors

  • L. I. Vergara

    • University of Tennessee
  • R. C. Rai

    • University of Tennessee
  • J. Cao

    • University of Tennessee
  • S. Brown

    • University of Tennessee
  • J. L. Musfeldt

    • University of Tennessee
  • D. J. Singh

    • Oak Ridge National Laboratory
  • G. Lawes

    • Wayne State University
  • N. Rogado

    • DuPont Central Research and Development
  • R. J. Cava

    • Princeton University
  • X. Wei

    • Florida State University