Magnetic order and lattice anomalies in the J$_1$-J$_2$ model system VOMoO$_4$

ORAL

Abstract

High resolution x-ray and neutron powder diffraction measurements were performed on polycrystalline VOMoO$_4$. Below $\simeq 40$ K the system orders in a simple N\'eel antiferromagnetic state (propagation vector $\vec{k}=0$), indicating a dominant role of the nearest-neighbor interactions. The order is three dimensional but the reduced saturated magnetic moment $m$ of 0.41 (1) $\mu_B/V^{4+}$ at 2 K indicates strongly 2D character and enhanced quantum fluctuations. On cooling, there is no evidence of a reduction of the crystal symmetry. However, neutron diffraction indicates an anomalous evolution of the lattice parameters, which can be related to the onset of magnetic correlations.

Authors

  • Alessandro Bombardi

    • Diamond Light Source
  • Laurent Chapon

    • ISIS-Rutherford Laboratory
  • Irene Margiolaki

    • ESRF
  • Claudio Mazzoli

    • ESRF
  • Sabine Ghontier

    • CNRS
  • Fabienne Duc

    • CNRS-Toulouse
  • Paolo G. Radaelli

    • ISIS, Rutherford Appleton Laboratory
    • ISIS Facility, Rutherford Appleton Laboratory, UK
    • ISIS-Rutherford Laboratory