NMR studies of quantum spin liquids using high magnetic fields: SrCu$_{2}$(BO$_{3})_{2}$ and BaCuSi$_{2}$O$_{6}$

ORAL

Abstract

We present the results of Nuclear Magnetic Resonance (NMR) experiments on the quasi-2D spin gap systems SrCu$_{2}$(BO$_{3})_{2}$ and BaCuSi$_{2}$O$_{6}$ in continuous magnetic fields H of up to 44 T. Using $^{11}$B spectra and spin-lattice relaxation times T$_{1}$ we explore the spin structure on the so-called 1/3 magnetization plateau of the Shastry-Sutherland model material SrCu$_{2}$(BO$_{3})_{2}$. In ancient Han purple - BaCuSi$_{2}$O$_{6}$ -- we observe with help of $^{29}$Si and $^{63,65}$Cu T$_{1}$ the closure of the singlet gap at H$_{c1}$ = 23.4 T down to temperatures T $\sim $ 40 mK. While entering the suggested Bose-Einstein Condensate phase for higher fields [M. Jaime \textit{et al}., Phys. Rev. Lett, \textbf{93}, 087203 (2004)] we discover dramatic changes in $^{29}$Si line shape suggesting incommensurate (and complicated) spin modulation in the ordered phase.

*work in Tallinn was supported by the Estonian Science Foundation grant 4931

Authors

  • Raivo Stern

    • NICPB, Akadeemia tee 23, EE12618 Tallinn, Estonia
  • I. Heinmaa

    • NICPB, Akadeemia tee 23, EE12618 Tallinn, Estonia
  • P. Kuhns

  • A. Reyes

  • W. Moulton

    • NHMFL, 1800 East Paul Dirac Dr., Tallahassee, FL 32310
  • M. Horvatic

  • C. Berthier

    • GHMFL-CNRS, 25 Avenue des Martyrs, F38042 Grenoble Cedex 9, France
  • C. Batista

  • M. Jaime

  • T. Kimura

    • NHMFL-LANL, Los Alamos, NM 87544
  • H. Dabkowska

  • B. D. Gaulin

    • Dept of Physics and Astronomy, McMaster University, Hamilton, Canada