GEC Student Excellence Award Finalist Presentation - Machine-learning-based prediction of plasma characteristics from optical emission spectra

ORAL

Abstract

Achieving consistent atomistic control in semiconductor plasma processing calls for real-time monitoring of the plasma conditions. While a simple and noninvasive diagnostic tool such as optical emission spectroscopy (OES) can be employed for such monitoring, interpreting the respective data to determine plasma characteristics is not an easy task. In this study, experimentally obtained OES data and plasma parameters obtained from particle-in-cell/Monte Carlo Collision (PIC/MCC) simulations as well as collisional-radiative model (CRM) simulations, combined with machine learning (ML) techniques were employed to predict plasma characteristics, including electron energy distribution functions (EEDF), from experimentally obtained OES data of radiofrequency-driven argon capacitively-coupled plasmas at various pressures (2-100 Pa). The use of several ML methods, including Multiple Kernel Ridge Regression, Random Forest, and Artificial Neural Networks, was investigated. This study first confirms that OES data of Ar discharges obtained from the coupled PIC/MCC-CRM simulations are in good agreement with measured OES data at low gas pressures. The inverse problem by the ML method also successfully predicts plasma parameters, including the EEDFs, from the measured OES data.

*1. Japan Ministry of Education, Culture, Sports, Science and Technology (MEXT)2. SFB1316 Project 'Transient atmospheric plasmas: from plasmas to liquids to solids'.3. Japan Society of the Promotion of Science (JSPS) Grants-in-Aid for Scientific Research(S) 15H05736 and (A) 21H044534. JSPS Core-to-Core Program JPJSCCA20190025. Osaka University International Joint Research Promotion Programs (Type A+)6. Casio Science Promotion Foundation7. Hungarian Office for Research, Development and Innovation (NKFIH) via the grant 134462.

Publication: 1. "First-principles simulation of optical emission spectra for low-pressure argon plasmas and its experimental validation," Fatima Jenina Arellano, Márton Gyulai, Zoltán Donkó, Peter Hartmann, Tsanko V. Tsankov, Uwe Czarnetzki, and Satoshi Hamaguchi, (2023) to be submitted.
2. "Machine learning-based prediction of plasma characteristics from optical emission spectra," Fatima Jenina Arellano, Zoltán Donkó, Peter Hartmann, Minoru Kusaba, Stephen Wu, Tsanko V. Tsankov, Uwe Czarnetzki, Ryo Yoshida, and Satoshi Hamaguchi, (2023) in preparation.

Presenters

  • Fatima Jenina Arellano

    • Osaka University, Japan

Authors

  • Fatima Jenina Arellano

    • Osaka University, Japan
  • Márton Gyulai

    • 1. Wigner Research Centre for Physics, Hungary 2. Eötvös Loránd University, Hungary
  • Zoltán Donkó

    • Wigner Research Centre for Physics
    • Wigner Research Centre for Physics, Hungary
    • 1. Wigner Research Centre for Physics, Hungary 2. Osaka University, Japan
  • Peter Hartmann

    • Wigner Research Centre for Physics, Hungary
  • Tsanko V Tsankov

    • Ruhr University Bochum, Germany
    • Ruhr-University Bochum, Faculty of Physics and Astronomy
  • Minoru Kusaba

    • The Institute of Statistical Mathematics, Japan
  • Stephen Wu

    • 1. The Institute of Statistical Mathematics, Japan 2. The Graduate University for Advanced Studies, Japan
  • Ryo Yoshida

    • The Institute of Statistical Mathematics, Japan and The Graduate University for Advanced Studies, Japan
  • Uwe Czarnetzki

    • Ruhr University Bochum, Germany
  • Satoshi Hamaguchi

    • Osaka University, Japan
    • Osaka University