Precise β-Decay Measurements of Long-Lived Fission Product <sup>111</sup>Ag

ORAL

Abstract

Our understanding of the fragment mass distributions following fission impacts many applications, including reactor-neutrino studies, nuclear forensics, and stockpile stewardship science. The γ-ray emissions following the β- decay of fission products provide a reliable signature that is often used to identify relative yields and distributions from fission. However, the uncertainties in the existing nuclear data for γ-ray intensities and β-decay branching ratios for some of the isotopes used in these applications range from 5-35%, which propagates to significant error contributions in fission-chain yield calculations. To address this issue, we have developed an experimental approach to precisely measure γ-ray branching ratios following the decay of long-lived fission products. We have identified 111Ag as vital isotope where the data can be significantly improved, and we prepared radioactive samples from the CARIBU facility for measurement with our established detection system at Texas A&M University. We will present high-precision results of absolute γ-ray intensities from the recent measurement of 111Ag, which were measured to ≤ 1%.

*This work is funded in part by the U.S. Department of Energy by the U.S. Department of Energy National Nuclear Security Administration through the Stewardship Science Graduate Fellowship as of September 1st, 2024.This work was performed in part under the auspices of the U.S. Department of Energy by the U.S. Department of Energy National Nuclear Security Administration through the Nuclear Science and Security Consortium under Award Nos. DE- NA0003180 and DE-NA0003996. The project was funded by the U.S. Department of Energy, National Nuclear Security Administration, Office of Defense Nuclear Nonproliferation Research and Development (DNN R&D).This work was performed in part under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. Lawrence Livermore National Security, LLC.

Presenters

  • Isabel E Hernandez

    • UC Berkeley

Authors

  • Isabel E Hernandez

    • UC Berkeley
  • Kay Kolos

    • Lawrence Livermore National Laboratory
  • Daniel E Hoff

    • Lawrence Livermore National Laboratory
  • Nicholas David Scielzo

    • Lawrence Livermore National Laboratory
  • Victor Iacob

    • Texas A&M University College Station
  • Dan G. Melconian

    • Texas A&M University College Station
  • Shree K Neupane

    • Lawrence Livermore National Laboratory
  • Daniel P Burdette

    • Argonne National Laboratory
  • Khushi Bhatt

    • Argonne National Laboratory
  • Jason Allan Clark

    • Argonne National Laboratory
  • Biying Liu

    • Notre Dame
    • University of Notre Dame
  • Brenden Longfellow

    • Lawrence Livermore National Laboratory
  • Peter Mueller

    • Argonne National Laboratory
  • Claus M Müller-Gatermann

    • Argonne National Laboratory
    • ANL
  • Andrea L Richard

    • Ohio University
    • Facility for Rare Isotope Beams; Department of Physics and Astronomy, Ohio University
  • D. Santiago-Gonzalez

    • Argonne National Laboratory
  • Guy Savard

    • Argonne National Laboratory
  • Anton P Tonchev

    • Lawrence Livermore National Laboratory
  • Adrian A. Valverde

    • Argonne National Laboratory
  • Louis Varriano

    • University of Washington