$^{239}$Pu Cumulative Fast Fission Product Yield Analysis

ORAL

Abstract

Precise integral measurement of fast neutron-induced fission product yields for various actinides is of high interest for applied nuclear science. The goal of this effort is to improve uncertainties in fission product yield values of $^{239}$Pu. Fission was induced in a pure $^{239}$Pu ($>99\%$) target using the Godiva-IV critical assembly in burst mode. The irradiated sample was transferred to a high-resolution $\gamma$-ray detector within 45 minutes. $\gamma$-ray list mode data was collected from 45 minutes to 1 week after the irradiation. $\gamma$-ray spectroscopy was performed to analyze the time dependent $\gamma$-ray yields using an automated peak search algorithm to identify isotopes by their decay $\gamma$-ray energy and half-life. The initial activity for each isotope identified was used to calculate their fission product yield.

*This work was funded by the Office of Defense Nuclear Nonproliferation Research and Development within the U.S. DOE - NNSA. This work was performed under the auspices of the U.S. DOE by LLNL under Contract DE-AC52-07NA27344. The National Criticality Experiments Research Center (NCERC), utilized in this work, is supported by the U.S. DOE Nuclear Criticality Safety Program, funded and managed by the NNSA for the DOE.

Authors

  • Aaron S. Tamashiro

    • Oregon State Univ
  • C.J. Palmer

    • Oregon State Univ
  • Jason T Harke

    • Lawrence Livermore Natl Lab
    • Lawrence Livermore National Laboratory, USA
  • Sean Burcher

    • Lawrence Livermore Natl Lab
    • University of Tennessee
  • S.W. Padgett

    • Lawrence Livermore Natl Lab
  • G. Slavik

    • Lawrence Livermore Natl Lab
  • N. Harward

    • Lawrence Livermore Natl Lab
  • N. Gharibyan

    • Lawrence Livermore Natl Lab
  • R. Henderson

    • Lawrence Livermore Natl Lab
  • B. Pierson

    • Pacific Northwest Natl Lab
  • L. Greenwood

    • Pacific Northwest Natl Lab
  • J. Goda

    • Los Alamos Natl Lab
  • D. Hayes

    • Los Alamos Natl Lab
  • J.A. Bounds

    • Los Alamos Natl Lab