Measurement of Short-Lived Fission Product Yields for $^{237}$Np via $\gamma$-ray Spectroscopy

ORAL

Abstract

Accurate fission product yields (FPYs) for neutron-induced fission of $^{237}$Np are important for applied nuclear science. The yields of short-lived fission products $(t_{1/2}$ $\lesssim$ hours$)$ are of particular interest, and are experimentally challenging to measure. High-resolution $\gamma$-ray spectroscopy can be used to determine the amount of various fission fragments produced by the unique $\gamma$-ray signatures of their decay, and does not require time-consuming chemical separation processes. Samples of $^{237}$Np have been irradiated in the Godiva-IV critical assembly, and then measured in a $\gamma$-ray counting setup for approximately 7 days. Hundreds of unique $\gamma$-rays were observed, allowing for the measurement of FPYs for many short-lived isotopes.

*This work was funded by the Office of Defense Nuclear Nonproliferation Research and Development within the U.S. DOE - NNSA. This work was performed under the auspices of the U.S. DOE by LLNL under Contract DE-AC52-07NA27344. The National Criticality Experiments Research Center (NCERC), utilized in this work, is supported by the U.S. DOE Nuclear Criticality Safety Program, funded and managed by the NNSA for the DOE.

Authors

  • Sean Burcher

    • Lawrence Livermore Natl Lab
    • University of Tennessee
  • J.T. Harke

    • Lawrence Livermore Natl Lab
  • S.W. Padgett

    • Lawrence Livermore Natl Lab
  • N. Gharibyan

    • Lawrence Livermore Natl Lab
  • N. Howard

    • Lawrence Livermore Natl Lab
  • K. Roberts

    • Lawrence Livermore Natl Lab
  • G. Slavik

    • Lawrence Livermore Natl Lab
  • P. Zhao

    • Lawrence Livermore Natl Lab
  • A.S. Tamashiro

    • Oregon State University
  • B.D. Pierson

    • Pacific Northwest Natl Lab
  • L. Greenwood

    • Pacific Northwest Natl Lab
  • J. Goda

    • Los Alamos Natl Lab
  • D. Hayes

    • Los Alamos Natl Lab
  • J. Hutchinson

    • Los Alamos Natl Lab
  • J. Walker

    • Los Alamos Natl Lab