Precision $\beta $-decay branching ratio measurements for long-lived fission products.

ORAL

Abstract

Nuclear data for fission products are used to determine fission-product yields, which impact nuclear applications. Many branching ratio measurements of long-lived fission products (t$_{\mathrm{1/2~}}$\textgreater 1d) suffer from high uncertainties, which contribute to the uncertainties in the determined fission yields. We developed a new experimental method to precisely (\textasciitilde 1{\%} precision) measure the~$\gamma $-ray branching ratios in the~$\beta $~decay of long-lived fission products. The approach involves production of a pure fission-product sample at the CARIBU facility at ANL on an ultra-thin carbon foil and a subsequent decay measurement with a 4$\pi $~gas proportional counter and a meticulously-calibrated high-purity germanium (HPGe) detector at TAMU. We will present results for~$^{\mathrm{95}}$Zr/$^{\mathrm{95}}$Nb,~$^{\mathrm{147}}$Nd, and$^{\mathrm{156}}$Eu.

*This work was performed under contract DE-AC52-07NA27344 (LLNL), DE-AC02-06CH11357 (ANL), DE-FG03-93ER40773 (TAMU), DE-AC0376SF0098 (UC), and supported by NNSA under the Funding Opportunity Announcement LAB 17-1763.

Authors

  • Miguel Bencomo

    • LLNL
  • Karolina Kolos

    • LLNL
  • Nicholas D Scielzo

    • LLNL
  • Wei Jia Ong

    • LLNL
  • Mark A Stoyer

    • LLNL
  • Anton P Tonchev

    • LLNL
  • Mary T Burkey

    • LLNL
  • Dan Melconian

    • TAMU
  • Victor E Iacob

    • TAMU
  • John C Hardy

    • TAMU
  • Jason A Clark

    • ANL
  • Matthew Gott

    • ANL
  • Daniel Santiago-Gonzalez

    • ANL
  • Guy Savard

    • ANL
  • Adrian Valverde

    • ANL
  • Xinliang Yan

    • ANL
  • Brian Champine

    • UC Berkeley
  • Tyler Nagel

    • UC Berkeley
  • Eric B Norman

    • UC Berkeley
  • Amber M Hennessy

    • UC Irvine
  • Rodney Orford

    • LBNL
  • Dwaipayan Ray

    • Univ. of Manitoba
  • Louis Varriano

    • Univ. of Chicago
  • Graeme Morgan

    • LSU
  • Shaofei Zhu

    • BNL