Energy Dependence of Fission Product Yields from $^{235}$U, $^{238}$U and $^{239}$Pu for Incident Neutron Energies Between 0.5 and 14.8 MeV

ORAL

Abstract

The energy dependence of a number of cumulative fission product yields (FPY) have been measured using quasi- monoenergetic neutron beams for three actinide targets, $^{235}$U, $^{238}$U and $^{239}$Pu, between 0.5 and 14.8 MeV. The FPYs were measured by a combi- nation of fission counting using specially designed dual-fission chambers and -ray counting. Each dual-fission chamber is a back-to-back ioniza- tion chamber encasing an activation target in the center with thin de- posits of the same target isotope in each chamber. This method allows for the direct measurement of the total number of fissions in the activa- tion target with no reference to the fission cross-section, thus reducing uncertainties. γ-ray counting of the activation target was performed on well-shielded HPGe detectors over a period of 2 months post irradiation to properly identify fission products. Reported are absolute cumulative fission product yields for incident neutron energies of 0.5, 1.37, 2.4, 3.6, 4.6 and 14.8 MeV. New data in the second chance fission region of 5.5 - 9 MeV are included.

*Work performed for the U.S. Department of Energy by Los Alamos National Security, LLC under contract DE-AC52-06NA25396.

Authors

  • Matthew Gooden

    • Los Alamos Natl Lab
  • Todd Bredeweg

    • Los Alamos National Laboratory
  • Malcolm Fowler

    • Los Alamos National Laboratory
  • David Vieira

    • Los Alamos National Laboratory
  • Jerry Wilhelmy

    • Los Alamos National Laboratory
  • Anton Tonchev

    • Lawrence Livermore National Laboratory
  • Mark Stoyer

    • Lawrence Livermore National Laboratory
  • Megha Bhike

    • Triangle Universities Nuclear Laboratory
  • Sean Finch

    • Triangle Universities Nuclear Laboratory
  • FNU Krishichayan

    • Triangle Universities Nuclear Laboratory
  • Werner Tornow

    • Triangle Universities Nuclear Laboratory