High-precision gamma-ray spectroscopy of 61Cu, an emerging medical isotope used in positron emission tomography

POSTER

Abstract

$^{61}$Cu ($t_{1/2}$ = 3.339h) is an important medical isotope used in positron emission tomography (PET) tumor hypoxia imaging scans; however, its beta-plus decay and the subsequent gamma decay of $^{61}$Ni has not been studied in over 30 years. Therefore, high quality decay data of $^{61}$Cu is desired to determine the overall dose delivered to a patient. In this study, $^{61}$Cu was produced at the University of Wisconsin - Madison cyclotron and then assayed using the Gammasphere array at Argonne National Laboratory. Consisting of 70 Compton-suppressed high-purity germanium (HPGe) detectors, Gammasphere provides precise decay data that exceeds that of previous $^{61}$Cu studies. $\gamma$-ray singles and coincident data were recorded and then analyzed using Radware gf3m software. Through $\gamma$-$\gamma$ coincidence techniques, new $\gamma$-ray transitions were identified and high precision determination of $\gamma$-ray intensities were made. These modifications and additions to the current decay scheme will be presented, and their impact on the resulting does estimates will be discussed.

*DOE Isotope Program is acknowledged for funding ST5001030. Work supported by the U.S. DOE under Grant No. DE-FG02-94ER40848 and Contract Nos. DE-AC02-98CH10946 and DE-AC02-06CH11357 and by the Science Undergraduate Laboratory Internship Program (SULI).

Authors

  • N. Nelson

    • Univ of Wisconsin, Madison
  • P. Ellison

    • Univ of Wisconsin, Madison
  • R. Nickles

    • Univ of Wisconsin, Madison
  • E. McCutchan

    • Brookhaven National Laboratory
  • A. Sonzogni

    • Brookhaven National Laboratory
  • S. Smith

    • Brookhaven National Laboratory
  • J. Greene

    • Argonne National Laboratory
  • M. Carpenter

    • Argonne National Laboratory
  • S. Zhu

    • Argonne National Laboratory
  • C. Lister

    • Univ of Massachusetts, Lowell
  • K. Moran

    • Univ of Massachusetts, Lowell