Using the 152Sm(p,3n)150Eu* Reaction as a Means to a Clean 150Gd target

ORAL

Abstract

As part of an ongoing program to measure direct neutron cross sections on radioactive targets, we have been investigating the feasibility of making a clean 150Gd target - a long-lived alpha-emitter of interest for stockpile stewardship - by making isomeric 150Eu, which decays to 150Gd with an 89{\%} branching ratio. In the first part of this study, the 152Sm(p,3n) reaction was studied at several energies ranging from 19-27 MeV, using an array of five clover Ge detectors to look at the relative population of the ground state ($\tau _{1/2}$ = 36.9 years) and the isomer ($\tau _{1/2}$ = 12 hour) of 150Eu. In the second experiment, we bombarded a thicker 152Sm target at 25 MeV and measured the delayed gamma rays from the ground state and isomer to get an absolute production yield. Preliminary results from these studies will be presented including a tentative excitation function.

*This work was performed under the auspices of the US Department of Energy by Lawrence Berkeley National Laboratory under contract D-ACO2-05CH11231 and NNSA Grant NA0078, and by Lawrence Livermore National Laboratory under contract W-7405-ENG-48.

Authors

  • B. Barquest

  • J. Cerny III

  • C. Jewett

    • LBNL \& UC Berkeley
  • D. Bleuel

  • M.A. McMahan

    • LBNL
  • L. Ahle

  • L. Bernstein

  • J. Burke

    • LLNL