Light dressing of excitonic states in monolayer WS<sub>2</sub>

ORAL

Abstract

Monolayer transition-metal dichalcogenides (TMDs) offer a novel platform of optoelectronic devices through their unique excitonic properties. Here, we perform optical transient absorption spectroscopy on monolayer tungsten disulfide (WS2) under an intense mid-infrared field, and observe a significant (more than a hundred meV) transient tuning of excitonic absorption. Experimentally, mid-infrared pulses (4 um, 100 fs, 0.2 V/nm) induce virtual 1s-np intraexcitonic transitions, and the resulting light-dressing effect is manifested in the optical absorption spectra (500-900 nm), featuring an AC-Stark shift and truncated free-induction decay. Theoretical insights are obtained by analyzing a few-level system within Floquet theory, and also by numerically solving the time-dependent Schrödinger equation for the driven system. Our results demonstrate a new scheme for the ultrafast and enhanced control of the excitonic properties in monolayer TMDs.

*This work was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the AMOS program. F.L. was supported by a Terman Fellowship and startup funds from the Department of Chemistry at Stanford University. Y.K. acknowledges support from the Urbanek- Chodorow Fellowship from Stanford University. C.H. acknowledges support from the W. M. Keck Foundation and a Humboldt Research Fellowship.

Presenters

  • Yuki Kobayashi

    • Stanford University

Authors

  • Yuki Kobayashi

    • Stanford University
  • Christian Heide

    • Stanford University
  • Amalya C Johnson

    • Stanford University
  • Jiaojian Shi

    • Stanford University
  • Fang Liu

    • Stanford University
  • David A Reis

    • Stanford University
  • Tony F Heinz

    • Stanford University
  • Shambhu Ghimire

    • SLAC National Accelerator Laboratory