Measuring sub-femtosecond x-ray pulses with angular streaking

POSTER

Abstract

The recent development of sub-femtosecond x-ray pulses from free-electron lasers has called for a high resolution measurement scheme to characterize such short pulses and the electronic dynamics they induce. The angular streaking technique exploits the phase-dependent momentum shift experienced by the photoelectrons ionized by x-ray pulses in the presence of a circularly polarized streaking laser field. We present a method to extract the temporal and spectral profiles of an electronic wavepacket produced by x-ray ionization from the photoelectron momentum distribution. We use this method to demonstrate the attosecond operation of a soft x-ray FEL, and study attosecond electron dynamics in x-ray photoionization.

*This work was supported by US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Chemical Sciences, Geosciences, and Biosciences Division; DOE, Office of Science, BES (DE-AC02-76SF00515); DOE, Office of Science, BES, Scientific User Facilities, Accelerator and Detector Research Division Field Work Proposal (100317); National Science Foundation Grant (PHY-1535215).

Authors

  • Siqi Li

    • SLAC National Accelerator Laboratory
  • P. Bucksbaum

    • SLAC National Accelerator Laboratory
  • E. Champenois

    • SLAC National Accelerator Laboratory
  • J. Cryan

    • SLAC National Accelerator Laboratory
  • T. Driver

    • SLAC National Accelerator Laboratory
  • J. Duris

    • SLAC National Accelerator Laboratory
  • R. Coffee

    • SLAC National Accelerator Laboratory
  • A. Gatton

    • SLAC National Accelerator Laboratory
  • Z. Huang

    • SLAC National Accelerator Laboratory
  • J. Knurr

    • SLAC National Accelerator Laboratory
  • M.F. Lin

    • SLAC National Accelerator Laboratory
  • J. MacArthur

    • SLAC National Accelerator Laboratory
  • T. Maxwell

    • SLAC National Accelerator Laboratory
  • M. Nantel

    • SLAC National Accelerator Laboratory
  • A. Natan

    • SLAC National Accelerator Laboratory
  • J. O'Neal

    • SLAC National Accelerator Laboratory
  • N. Shivaram

    • SLAC National Accelerator Laboratory
  • P. Walter

    • SLAC National Accelerator Laboratory
  • T. Wolf

    • SLAC National Accelerator Laboratory
  • A. Marinelli

    • SLAC National Accelerator Laboratory
  • M. Kling

    • Department of Physics, Ludwig-Maximilians-Universitat Munchen
  • P. Rosenberger

    • Department of Physics, Ludwig-Maximilians-Universitat Munchen
  • G. Hartmann

    • Institut fur Physik und CINSaT, Universitat Kassel
  • W. Helml

    • Max Planck Institute of Quantum Optics