Attosecond delay and angular asymmetry in plasmonic photoemission of C$_{60}$

POSTER

Abstract

We present a theory-experiment joint study of effects of the giant plasmon resonance of C$_{60}$ on photoionization angular asymmetry, phase and time delay. Phases of ionization amplitudes are utilized to compute Wigner-Smith delays and angular asymmetries of emissions from HOMO and HOMO-1 levels in time-dependent local density approximation (TDLDA) [1, 2], uncovering significant plasmon effects [3]. Electron momentum imaging spectroscopy is used to measure the photoelectron angular distribution asymmetry parameter at the plasmon that agreed well with TDLDA [3]. Preliminary results of our experiments using RABITT pump-probe metrology show promise of attosecond measurements of plasmon-driven delays to complement our predictions. * franck.lepine@univ-lyon1.fr ** himadri@nwmissouri.edu \\[4pt] [1] Madjet et al., JPB 41, 105101 (2008);\\[0pt] [2] Maurat et al., JPB 42, 165105 (2009);\\[0pt] [3] Barillot et al., (in review).

*Supported by the US NSF, CNRS, ANR.

Authors

  • T. Barillot

    • Institut Lumiere matiere, France
  • C. Cauchy

    • Institut Lumiere matiere, France
  • V. Loriot

    • Institut Lumiere matiere, France
  • C. Bordas

    • Institut Lumiere matiere, France
  • F. Lepine

    • Institut Lumiere matiere, France
  • P-A. Hervieux

    • Chimie des materiaux, France
  • M. Gisselbrecht

    • Lund University, Sweden
  • P. Johnsson

    • Lund University, Sweden
  • J. Laksman

    • Lund University, Sweden
  • E. Mansson

    • Lund University, Sweden
  • S. Sorensen

    • Lund University, Sweden
  • S. Canton

    • Lund University, Sweden
  • J. Dahlstrom

    • Stockholm University, Sweden.
  • M. Magrakvelidze

    • Northwest Missouri State University
  • H. Chakraborty

    • Northwest Missouri State University
  • G. Dixit

    • MBI, Berlin, Germany
  • M. Madjet

    • QEERI, Doha, Qatar