Atom Trap Trace Analysis Reaches a Part-per-quadrillion Sensitivity

ORAL

Abstract

A quadrillion is 10$^{15}$. This is how many argon atoms one has to sift through in order to find just one atom of the radioactive isotope $^{39}$Ar. Atom Trap Trace Analysis (ATTA), a MOT-based atom counting method, is now able to unambiguously pick $^{39}$Ar out of a regular argon gas sample. The exceedingly rare $^{39}$Ar forms naturally in the environment by cosmic rays, decays with a half-life of 270 years, and is an ideal tracer to study ocean circulation or groundwater flow over the past few hundred years. In an ATTA apparatus, only $^{39}$Ar atoms are selectively captured by the MOT, appear as a bright dot, and can be counted one atom at a time using a sensitive camera. This work constitutes a major breakthrough in analytical capability, and promises to enable a wide range of applications in physics as well as earth sciences.

*Support comes from DOE, Office of Nuclear Physics, under contract DEAC02-06CH11357; and from NSF, Division of Earth Sciences, under Award No. EAR-0651161.

Authors

  • Wei Jiang

    • Physics Div, Argonne National Lab
    • Argonne National Lab, Illinois 60439, USA
  • William Williams

    • Physics Div, Argonne National Lab
    • Argonne National Lab, Illinois 60439, USA
  • K. Bailey

    • Argonne National Laboratory
    • Physics Div, Argonne National Lab
    • Argonne National Lab, Illinois 60439, USA
    • Argonne National Lab
  • Andrew Davis

    • Univ of Chicago
    • Univ of Chicago, USA
  • Shuiming Hu

    • Hefei National Lab, Univ of Sci \& Tech of China
    • USTC, Hefei, China
  • Zheng-Tian Lu

    • Physics Division, Argonne National Laboratory; The Department of Physics and Enrico Fermi Institute, The University of Chicago
    • Argonne National Laboratory
    • Physics Div, Argonne National Lab, Univ of Chicago
    • Argonne National Lab, Illinois 60439, USA
  • T.P. O'Connor

    • Argonne National Laboratory
    • Physics Div, Argonne National Lab
    • Argonne National Lab, Illinois 60439, USA
    • Argonne National Lab
  • Roland Purtschert

    • Univ of Bern
    • Univ of Bern, Bern, Switzerland
  • Neil Sturchio

    • Univ of Chicago
    • Univ of Illinois, Chicago, USA
  • Yun Sun

    • Hefei National Lab, Univ of Sci \& Tech of China
    • USTC, Hefei, China
  • P. Mueller

    • Argonne National Laboratory
    • Physics Div, Argonne National Lab
    • Argonne National Lab, Illinois 60439, USA
    • Argonne National Lab